The present paper proposes a new method for constructing polyphase asymmetric zero-correlation zone (A-ZCZ) sequence sets. The proposed method can generate A-ZCZ sequence sets that cannot be obtained from methods proposed by other researchers and is a generalized version of our previously proposed method. An A-ZCZ sequence set can be regarded as a ZCZ sequence set. The newly obtained A-ZCZ sequence sets include quasi-optimal ZCZ sequence sets of which the zero-cross-correlation zone (ZCCZ) length between different sequence subsets is larger than the mathematical upper bound of conventional ZCZ sequence sets. A new method for extending the A-ZCZ sequence sets is also presented in the present paper.