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Effective chirality discrimination via dissipation dynamics

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Abstract

In this paper, we propose a protocol to distinguish chiral molecules using dissipation dynamics. The physical model is based on a four-level structure with a ground level, a lower level, and two excited levels. Under the condition of large detuning, a chirality-selective transition from the ground level to a dressed state of two excited levels can be achieved, where only the left-handed enantiomer can be exited to the dressed state. The left-handed enantiomer in the dressed state will couple with the cavity mode and evolve to the lower level with a photon creation. When the photon loss happens, the left-handed enantiomer cannot be excited to the dressed state again by absorbing the photon, thus remaining in the lower level. Then, the chiralities of the enantiomers can be distinguished by measuring their final states. We take 1,2-propanediol molecules as an example to demonstrate the protocol, where the difference of the populations of the lower level for the left- and right-handed enantiomer approaches unity in a relatively short operation time. Numerical simulation results show that the scheme is insensitive to the influence of the phase drift and frequency mismatch. Therefore, the protocol may provide an alternative approach for chirality discrimination.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China under Grant Nos. 11575045, 11874114, and 11674060, the Natural Science Funds for Distinguished Young Scholar of Fujian Province under Grant 2020J06011, and the Project from Fuzhou University under Grant JG202001-2.

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  1. Fujian Key Laboratory of Quantum Information and Quantum Optics, Fuzhou University, Fuzhou, 350108, China

    Wei-Wei Ding, Yi-Hao Kang, Yang Liu, Bi-Hua Huang & Yan Xia

  2. Department of Physics, Fuzhou University, Fuzhou, 350108, China

    Wei-Wei Ding, Yi-Hao Kang, Yang Liu, Bi-Hua Huang & Yan Xia

  3. Department of Electronic Information Engineering, Maynooth International Engineering College, Fuzhou University, Fuzhou, 350108, China

    Zhe-Ping Lin

  4. Department of Physics, Harbin Institute of Technology, Harbin, 150001, China

    Yi-Hao Kang & Jie Song

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Ding, WW., Lin, ZP., Kang, YH. et al. Effective chirality discrimination via dissipation dynamics. Quantum Inf Process 22, 350 (2023). https://doi.org/10.1007/s11128-023-04109-8

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