Abstract
Radon concentration was continuously monitored in a horizontal dead-end gallery near Vyhne (Central Slovakia) from October 2005 to April 2008. Hourly average of radon varied from 2800 to 10 500 Bq/m3. Temporal variation of radon, which contains periodic and non-periodic signals, spans variation of annual to diurnal scale. Time series of radon were analyzed together with meteorological parameters. The annual variation of radon seems to be connected with the annual variation of atmospheric pressure. The amplitude and shape of diurnal variation of radon changed during the year and is correlated with corresponding changes in the daily amplitude of atmospheric pressure.
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References
Steinitz G, Begin ZB, Gazit-Yaari N (2003) Statistically significant relation between radon flux and weak earthquakes in the Dead Sea rift valley. Geology 31:505–508. https://doi.org/10.1130/0091-7613(2003)031%3c0505:SSRBRF%3e2.0.CO;2
Cigolini C, Laiolo M, Coppola D (2007) Earthquake–volcano interactions detected from radon degassing at Stromboli (Italy). Earth Planet Sci Lett 257:511–525. https://doi.org/10.1016/j.epsl.2007.03.022
Briestenský M, Thinová L, Stemberk J, Rowberry MD (2011) The use of caves as observatories for recent geodynamic activity and radon gas concentrations in the Western Carpathians and Bohemian Massif. Radiat Prot Dosim 145:166–172. https://doi.org/10.1093/rpd/ncr080
Neri M, Giammanco S, Ferrera E, Patanè G, Zanon V (2011) Spatial distribution of soil radon as a tool to recognize active faulting on an active volcano: the example of Mt. Etna (Italy). J Environ Radioactiv 102:863–870. https://doi.org/10.1016/j.jenvrad.2011.05.002
Barbosa SM, Donner RV, Steinitz G (2015) Radon applications in geosciences – Progress & perspectives. Eur Phys J Special Topics 224:597–603. https://doi.org/10.1140/epjst/e2015-02393-y
Sainz C, Rábago D, Celaya S, Fernández E, Quindós J, Quindós L (2018) Continuous monitoring of radon gas as a tool to understand air dynamics in the cave of Altamira (Cantabria, Spain). Sci Total Environ 624:416–423. https://doi.org/10.1016/j.scitotenv.2017.12.146
Ballesteros D, Llana-Fúnez S, Meléndez-Asensio M, Fuente Merino I, Sainz C, Quindós L, DeFelipe I (2021) Radon concentration in caves as a proxy for tectonic activity in The Cantabrian Mountains (Spain). Acta Carsologica 50(1):165–182. https://doi.org/10.3986/ac.v50i1.7795
Muramatsu H, Tashiro Y, Hasegawa N, Misawa C, Minami M (2002) Seasonal variations of 222Rn concentrations in the air of tunnel located in Nagano city. J Environ Radioactiv 60:263–374. https://doi.org/10.1016/S0265-931X(01)00085-6
Barbosa SM, Zafrir H, Malik U, Piatibratova O (2010) Multi-year to daily radon variability from continuous monitoring at the Amram tunnel, southern Israel. Geophys J Int 182:829–842. https://doi.org/10.1111/j.1365-246X.2010.04660.x
Gregorič A, Zidanšek A, Vaupotič J (2011) Dependance of radon levels in Postojna Cave on outside air temperature. Nat Hazards Earth Syst Sci 11:1523–1528. https://doi.org/10.5194/nhess-11-1523-2011
Mentes G, Eper-Pápai I (2015) Investigation of temperature and barometric pressure variation effects on radon concentration in the Sopronbánfalva Geodynamic Observatory. Hungary J Environ Radioactiv 149:64–72. https://doi.org/10.1016/j.jenvrad.2015.07.015
Tchorz-Trzeciakiewicz DE, Parkitny T (2015) Radon as a tracer of daily, seasonal and spatial air movements in the Underground Tourist Route “Coal Mine” (SW Poland). J Environ Radioactiv 149:90–98. https://doi.org/10.1016/j.jenvrad.2015.07.006
Briestenský M, Ambrosino F, Smetanová I, Thinová L, Šebela S, Stemberk J, Pristašová L, Pla C, Benavente D (2022) Radon in dead-end caves In Europe. J Cave Karst Stud 84:41–50. https://doi.org/10.4311/2021es0101
Hakl J, Csige I, Hunyadi I (1996) Radon transport in fractured porous media – experimental study in caves. Environ Int 22:S433–S437. https://doi.org/10.1016/S0160-4120(96)00143-2
Garavaglia M, Braitenberg C, Zadro M (1998) Radon monitoring in a cave of North-Eastern Italy. Phys Chem Earth 23:949–952. https://doi.org/10.1016/S0079-1946(98)00125-6
Eff-Darwich A, Martín-Luis C, Quesada M, de la Nuez J, Coello J (2002) Variations on the concentration of 222Rn in the subsurface of the volcanic island of Tenerife. Canary Islands Geophys Res Lett 29:2069. https://doi.org/10.1029/2002GL015387
Zafrir H, Barbosa SM, Malik U (2013) Differentiation between the effect of temperature and pressure on radon within the subsurface geological media. Radiat Meas 49:39–56. https://doi.org/10.1016/j.radmeas.2012.11.019
Whittlestone S, James J, Barnes C (2003) The relationship between local climate and radon concentrations in the Temple of Baal, Jenolan Caves, Australia. Helictite 38:39–44
Perrier F, Richon P, Gautam U, Tiwari RD (2007) Seasonal variations of natural ventilation and radon-222 exhalation in a slightly rising dead-end tunnel. J Environ Radioactiv 97:220–235. https://doi.org/10.1016/j.jenvrad.2007.06.003
Gregorič A, Vaupotič J, Šebela S (2014) The role of cave ventilation in governing cave air temperature and radon levels (Postojna Cave, Slovenia). Int J Climatol 34:1488–1500. https://doi.org/10.1002/joc.3778
Trique M, Richon P, Perrier F, Avouac JP, Sabroux JC (1999) Radon emanation and electric potential variations associated with transient deformation near Reservoir lakes. Nature 399:137–141. https://doi.org/10.1038/20161
Kies A, Massen F, Tosheva Z (2002) Influence of variable stress on underground radon concentration. Geofísica Int 41:325–329
Shirokov IA, Rosa K, Kubačková L, Hudec P (1977) The Tidal station of the Geophysical Institute of the Slovak Academy of Sciences in Vyhne. Contrib Geophys Inst Slovak Acad Sci 7:209–215
Brimich L, Bednárik M, Bezák V, Kohút I, Ban D, Eper-Pápai I, Mentes G (2016) Extensometric observation of Earth tides and local tectonic processes at the Vyhne station, Slovakia. Contrib Geophys Geodesy 46:75–90. https://doi.org/10.1515/congeo-2016-0006
Konečný V, Lexa J, Halouzka R, Dublan L, Šimon L, Stolár M, Nagy A, Polák M, Vozár J, Havrila M, Pristaš J (1998) Geologická mapa Štiavnických vrchov a Pohronského Inovca (Štiavnický stratovulkán)/Geological map of the region Štiavnické vrchy Mts. and Pohronský Inovec Mts. (Štiavnica stratovolcano) (1:50 000). Geological Survey of the Slovak Republic, Bratislava. ISBN: 80–85314–85–1 (in Slovak)
Konečný V, Lexa J., Halouzka R, Hók J, Vozár J, Dublan L, Nagy A, Šimon L, Havrila M, Ivanička J, Hojstričová V, Miháliková A, Vozárová A, Konečný P, Kováčiková M, Filo M, Marcin D, Klukanová A, Liščák P, Žáková E (1998) Vysvetlivky ku geologickej mape Štiavnických vrchov a Pohronského Inovca (Štiavnický stratovulkán)/ Explanation to the geological map of the Štiavnické vrchy Mts. and Pohronský Inovec Mts. (Štiavnica stratovolcano) (1:50,000). Geological Survey of the Slovak Republic, Bratislava: 1–473 (in Slovak)
Smetanová I, Holý K, Briestenský M, Zelinka J, Omelka J (2013) Continual Monitoring of Radon in Underground Environments in Slovakia. In: Kovács T, Somlai J, Ferenc F (Eds.): VII. Hungarian Radon Forum and Radon in Environment Satellite Workshop. University of Pannonia, Social Organization for Radioecological Cleanliness, Hungarian Biophysical Society, Veszprém 16.-17.5. 2013, Pannonian University Press: 161-170. ISBN 978-615-5044-91-5
Papastefanou C (2007) Measuring radon in soil gas and groundwaters: a review. Ann Geophys 50:569–578. https://doi.org/10.4401/ag-3070
Sýkora I, Ješkovský M, Janík R, Holý K, Chudý I, Povinec PP (2008) Low-level single and coincidence gamma-ray spectrometry. J Radioanal Nucl Ch 276:779–787. https://doi.org/10.1007/s10967-008-0632-8
Morawska L, Phillips CR (1991). In: Kay JG, Keller GE, Miller JF (eds) Indoor air pollution: radon, bioaerosols and VOCs. Lewis Publishers, Michigan, pp 201–215
Holý K, Sýkora I, Chudý M, Polášková A, Fejda J, Holá O (1995) Radionuclide content in some building materials and their radon exhalation. J Radioanal Nulc Chem Lett 199:251–263
Richon P, Perrier F, Sabroux J-C, Trique M, Ferry C, Voisin V, Pili E (2005) Spatial and time variations of radon-222 concentration in the atmosphere of a dead-end horizontal tunnel. J Environ Radioactiv 78:179–198. https://doi.org/10.1016/j.jenvrad.2004.05.001
Fuyioshi R, Morimoto H, Sawamura S (2002) Investigation of soil radon variation during the winter months in Sapporo, Japan. Chemosphere 47:369–373. https://doi.org/10.1016/S0045-6535(01)00310-1
Box G, Jenkins G, Reinsel G (2008) Time series analysis: Forecasting and control. New Jersey: John Wiley & Sons Inc. (fourth edition). ISBN: 978-1-118-61919-3
Daniel J, Lučivjanský L, Stercz M (1996) Geochemical atlas of Slovakia, part IV. Natural rock radioactivity. Geological survey of Slovak Republic, Bratislava
International Atomic energy agency (2003) Guidelines for radioelement mapping using gamma ray spectrometry data. IAEA Vienna
Acknowledgements
The authors would like to thank Dr. Miroslav Ješkovský from the Faculty of Mathematics, Physics and Informatics, Comenius University in Bratislava for the measurements of mass activities.
Funding
This work was supported by the Slovak Research and Development Agency of Ministry of Education, Science, Research and Sport of the Slovak Republic (project APVV: SK-PT-18–0015), the Scientific Grant Agency of Ministry of Education, Science, Research and Sport of the Slovak Republic (VEGA project 2/0015/21), and Fundação para a Ciência e Tecnologia (FCT) in the framework of the bilateral Portugal-Slovakia project RADCAMIN.
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Smetanová, I., Barbosa, S.A., Vďačný, M. et al. The effect of environmental parameters on radon concentration measured in an underground dead-end gallery (Vyhne, Slovakia). J Radioanal Nucl Chem 332, 1733–1742 (2023). https://doi.org/10.1007/s10967-023-08884-7
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DOI: https://doi.org/10.1007/s10967-023-08884-7